2010–present: film success and beyond
On 21 October 2010, Peter Jackson announced Armitage was cast as Thorin Oakenshield in the three-film production of The Hobbit. All three films were released in December, starting with The Hobbit: An Unexpected Journey in 2012, The Hobbit: The Desolation of Smaug in 2013 and The Hobbit: The Battle of the Five Armies in 2014. Armitage thought it was a wonderful opportunity, as he grew up reading the book. Coincidentally, one of his first stage roles was playing an elf in a production of The Hobbit at the Alex Theatre in Birmingham. He describes the character of Thorin as being complex and flawed, "somebody that had doubts and that had fears, and there was a gentle side to him and a very perhaps lonely side to him." He notes the scene with Balin in Bag End shows the character's inner sensitivity and fear of failure, "failing where his father and his grandfather had failed as well."
After filming had been completed on The Hobbit, Armitage flew to Detroit, Michigan to film Into the Storm from July to September 2012. He starred as Gary Fuller, a high school vice principal and football coach with two teenage sons. The film from New Line was released in August 2014.
In March 2014, Armitage began the eight-week shoot of an adaptation of Bernard Hare's memoir Urban Grimshaw and the Shed Crew in Leeds, UK. He played "Chop" (the author's nickname), an ex-social worker, drunk and drug addict in Britain's lowerclass who befriends the hardened young delinquent Urban. Armitage explained his attraction to this role: "it ticks a few boxes for me: it"s based on a really interesting piece of literature, but also based on living people, who have been working with us on set." Urban and the Shed Crew premiered at the Leeds International Film Festival (LIFF) on 7 November 2015.
Armitage next appeared as John Proctor in The Old Vic's production of Arthur Miller's The Crucible. Directed by Yaël Farber and performed in the round, the play ran from 21 June to 13 September 2014. The production drew an unprecedented number of 5-star reviews and was a commercial success. For his performance, Armitage was awarded Best Leading Actor in a New Production of a Play by Broadway World:UK Awards 2014 and a Best Actor nomination for an Olivier Award. Due to worldwide demand to see the production, Digital Theatre captured the live performance to bring The Crucible to cinemas and for digital download. It was screened at cinemas on 4 and 7 December 2014 in the UK and Ireland, with further screenings in other selected territories in February and March 2015. Copyright issues prevented the film from being screened at North American cinemas. Digital Theatre made the digital download available worldwide on 17 March 2015.
In a September 2014 interview, Armitage revealed he would film his cameo role of King Oleron in Alice Through the Looking Glass in London after The Crucible closed. The film was released in May 2016.
Armitage spent four weeks in October 2014 filming Sleepwalker in the greater Los Angeles area. In this psychological thriller, Armitage plays Dr. Scott White, a senior MD at a sleep research center. Released on 4 February 2017.
DeLaurentiis Company tweeted on 13 January 2015 that Armitage was cast as Francis Dolarhyde in the TV production of Hannibal, written and co-produced by Bryan Fuller. Dolarhyde is a serial killer, a character type which Armitage had expressed interest in portraying. He filmed the series in Toronto, Canada from January to April, and the series aired from 4 June to 29 August 2015. Armitage appeared in the last six episodes of season 3, earning high praise, wide acclaim and several award nominations, including two wins.
After wrapping on Hannibal in late April 2015, Armitage joined his fellow Pilgrimage castmates who had already begun filming in Connemara, Ireland two weeks prior. He plays Sir Raymond De Merville, a 13th-century French Norman who is intent on foiling a group of monks escorting a sacred relic from Ireland to Rome. The cast and crew later moved to the Ardennes region of Belgium to complete filming, with Armitage wrapping one week earlier than the film wrap at the end of May.
News broke on 13 May 2015 that Armitage would star in Clearance, the first English language film by Finnish director Aku Louhimies and set to film in South Africa in November 2015. It is an action drama about a hardened mine expert named Ray (Armitage) and his pregnant partner (Naomie Harris) who are kidnapped in South Sudan.
In a June 2015 interview, Armitage mentioned his next projects included an Edith Wharton film and a true Irish tragic drama. Per agent David Higham, Bridget Cleary is likely the Irish drama.
On 12 July 2015, Armitage revealed he was about to start filming Brain on Fire in Vancouver, Canada. Subsequent news outlets provided more details about his role as "Big Man" Tom Cahalan, father of the protagonist in the true-life story of young journalist Susannah Cahalan's sudden descent into inexplicable madness and the eleventh-hour diagnosis by one doctor. Filming began 13 July 2015. Brain on Fire premiered at the Toronto International Film Festival (TIFF) on 14 September 2016.
Armitage landed the lead role of Daniel Miller in Berlin Station, an original spy series for Epix. His character, a cerebral analyst from Langley, is a newly anointed undercover CIA officer tasked with finding a mole in Berlin. Filmed in Berlin from November 2015 to April 2016, with some additional filming in the Canary Islands, the series premiered on Epix in the autumn of 2016.
On 13 July 2016, Roundabout Theatre Company announced Armitage was cast as Kenneth in the American premiere of Love, Love, Love by playwright Mike Bartlett. Love, Love, Love marks Armitage's first leading role in a theatrical play on an American stage. The off-Broadway play ran from 22 September to 18 December 2016 at the intimate Laura Pels Theater in New York City.
Armitage co-starred in the heist comedy Ocean's 8 (2018).
In February 2017, it was announced that Armitage had joined the cast of Julie Delpy's film My Zoe. In it he will play the role of James, the ex-husband of Delpy's character Isabelle. Their toxic marriage may be over but they are still in contact with each other as they co-parent their daughter Zoe. But when tragedy strikes this fractured family, Isabelle takes matters into her own hands. In February 2018, Armitage joined the cast of The Lodge, which began filming in early February. Armitage plays the leading role of Adam Price in Netflix's 2020 mystery thriller miniseries, The Stranger, which is based on the Harlan Coben novel of the same title. The series has been critically acclaimed, with a rating of 89% from Rotten Tomatoes.
In 2022, Armitage gave his first performance in a video game, appearing as the Daemon Prince Be'lakor in Creative Assembly's real-time strategy game Total War: Warhammer III. In October that year, Armitage's debut novel, Geneva, a thriller, was published by Audible. Armitage and former Spooks co-star Nicola Walker narrate the audiobook.